2-COLOR DYNAMIC LIGHT-SCATTERING
SEGRE PN, VANMEGEN W, PUSEY PN, SCHATZEL K, PETERS W
JOURNAL OF MODERN OPTICS
42: (9) 1929-1952 SEP 1995
Abstract:
The design, alignment and operation of improved two-colour
dynamic light scattering equipment which effectively
suppresses multiple scattering and allows the study of
the Brownian dynamics of optically turbid samples is
described. The technique operates by cross-correlating
scattered light of two different colours. With the
appropriate scattering geometry, only singly scattered
light contributes to the time-dependent part of the measured
intensity cross-correlation function thus allowing straightforward
interpretation of the data. To demonstrate the
performance of the instrument we have studied various
colloidal suspensions. Although dilute enough that free
diffusion of the particles can be assumed, the samples
ranged from quite transparent to distinctly turbid. We have
confirmed that the measured cross-correlation functions
accurately reflect only single scattering even in the
presence of strong multiple scattering.